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null (Ed.)Zinc-ion battery (ZIB) has been attracting extensive attention due to its high theoretical capacity, high safety, and low cost. However, the exploration of suitable cathode materials to host Zn ions remains a challenge, owing to the strong electrostatic interactions and large steric hindrance effects between Zn ion and host materials. Great efforts have been devoted to the optimization of the structure and electrochemical property of the cathode materials. In this review article, we summarize recent cathode-based strategies to address the issues of performance degradation and structural collapse of electrode materials within the context of microstructure design and ion/charge transport mechanism, and include a perspective to highlight the challenges and promises in the exploitation of cathode materials for further enhancement of the performance of ZIBs.more » « less
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He, Pingge; Chen, Shaowei (, ChemElectroChem)Abstract Vertically oriented graphene (VG) nanosheets exhibit unique structural characteristics, such as large accessible surface area, rich edges, high electrical conductivity, open network channels, and agglomeration resistance, for electrochemical energy‐storage applications (e. g., supercapacitors, lithium‐ion batteries, etc.). In this Review article, we summarize recent progress in the design and engineering of VG‐based electrodes for high‐performance electrochemical energy technologies within the context of energy‐storage mechanisms and charge‐transfer kinetics, and include a perspective to highlight the challenges and promises in the exploitation of vertically oriented two‐dimensional carbon nanostructures for further enhancement of the performance of electrochemical energy‐storage devices.more » « less
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